Absolute Rate Theory

The velocity (v) of the reaction S ® P is the rate of formation of P.

v = k [S] where k is the rate constant.

According to absolute rate theory the reaction actually progresses as follows:

S ® TS ® P were TS is the "transition state"

We define the activation energy (DG*) as the difference in free energy between S and TS, i.e.

DG* = GTS - GS

TS always has a higher free energy than S, so DG* is always positive.

As is the case for all DGs, DG* contains enthalpy and entropy components:

DG* = DH* - TDS*

The rate constant (k) for the reaction is a function of DG*:

k = Ce-DG*/RT or alternatively:

ln(k) = ln(C) - DG*/RT

where R and C are constants.